Steinmann J.L., Blomley E., Brosi M., Brundermann E., Caselle M., Hesler J.L., Hiller N., Kehrer B., Mathis Y.-L., Nasse M.J., Raasch J., Schedler M., Schonfeldt P., Schuh M., Schwarz M., Siegel M., Smale N., Weber M., Muller A.-S.
in Physical Review Letters, 117 (2016), 174802. DOI:10.1103/PhysRevLett.117.174802
© 2016 American Physical Society. Using arbitrary periodic pulse patterns we show the enhancement of specific frequencies in a frequency comb. The envelope of a regular frequency comb originates from equally spaced, identical pulses and mimics the single pulse spectrum. We investigated spectra originating from the periodic emission of pulse trains with gaps and individual pulse heights, which are commonly observed, for example, at high-repetition-rate free electron lasers, high power lasers, and synchrotrons. The ANKA synchrotron light source was filled with defined patterns of short electron bunches generating coherent synchrotron radiation in the terahertz range. We resolved the intensities of the frequency comb around 0.258 THz using the heterodyne mixing spectroscopy with a resolution of down to 1 Hz and provide a comprehensive theoretical description. Adjusting the electron’s revolution frequency, a gapless spectrum can be recorded, improving the resolution by up to 7 and 5 orders of magnitude compared to FTIR and recent heterodyne measurements, respectively. The results imply avenues to optimize and increase the signal-to-noise ratio of specific frequencies in the emitted synchrotron radiation spectrum to enable novel ultrahigh resolution spectroscopy and metrology applications from the terahertz to the x-ray region.